| 1 | Aurora (The Squires) |
| 2 | The Sultan (The Squires) |
| 3 | I Wonder (The Squires) |
| 4 | Mustang (The Squires) |
| 5 | I'll Love You Forever (The Squires) |
| 6 | (I'm A Man And) I Can't Cry (The Squires) |
| 7 | Hello Lonely Woman [Previously Unreleased Original Recording] |
| 8 | Casting Me Away From You [Previously Unreleased Original Recording] |
| 9 | 9. There Goes My Babe [Previously Unreleased Original Recording] |
| 10 | Sugar Mountain (Neil Young) |
| 11 | Nowadays Clancy Can't Even Sing [Previously Unreleased Original Demo Recording] [Mono] |
| 12 | Runaround Babe [Previously Unreleased Original Recording] [Mono] |
| 13 | The Ballad Of Peggy Grover [Previously Unreleased Original Recording] [Mono] |
| 14 | The Rent Is Always Due [Previously Unreleased Original Recording] [Mono] |
| 15 | Extra, Extra [Previously Unreleased Original Recording] [Mono] |
| 16 | Flying On The Ground Is Wrong (Neil Young) |
| 17 | Burned [Mono] |
| 18 | Out Of My Mind [Mono] |
| 19 | Down, Down, Down [Previously Unreleased Original Recording] |
| 20 | Kahuna Sunset [Mono] |
| 21 | Mr. Soul [Mono] |
| 22 | Sell Out [Previously Unreleased Song] [Mono] |
| 23 | Down To The Wire [Mono] |
| 24 | Expecting To Fly (Buffalo Springfield) |
| 25 | Slowly Burning [Previously Unreleased Unfinished Recording] |
| 26 | One More Sign |
| 27 | Broken Arrow (Buffalo Springfield) |
| 28 | I Am A Child |
| 29 | Everybody Knows This Is Nowhere (Neil Young) |
| 30 | The Loner |
| 31 | Birds (Neil Young) |
| 32 | What Did You Do To My Life? [Previously Unreleased Mix] |
| 33 | The Last Trip To Tulsa (Neil Young) |
| 34 | Here We Are In The Years |
| 35 | I've Been Waiting For You [Previously Unreleased Mix] |
| 36 | The Old Laughing Lady (Neil Young) |
| 37 | I've Loved Her So Long (Neil Young) |
| 38 | Sugar Mountain [Previously Unreleased Stereo Master] |
| 39 | Nowadays Clancy Can't Even Sing [Previously Unreleased Live Version] |
| 40 | Down By The River (Neil Young with Crazy Horse) |
| 41 | Cowgirl In The Sand (Neil Young with Crazy Horse) |
| 42 | Everybody Knows This Is Nowhere (Neil Young with Crazy Horse) |
| 43 | Sugar Mountain (Neil Young) |
| 44 | The Old Laughing Lady |
| 45 | Flying On The Ground Is Wrong-live (Neil Young) |
| 46 | On The Way Home [Live At The Riverboat 1969] [Previously Limited Release] |
| 47 | I've Loved Her So Long-live (Neil Young) |
| 48 | I Am A Child [Live At The Riverboat 1969] [Previously Limited Release] |
| 49 | 1956 Bubblegum Disaster (Neil Young) |
| 50 | The Last Trip To Tulsa [Live At The Riverboat 1969] [Previously Unreleased Live Version] |
| 51 | Broken Arrow-live (Neil Young) |
| 52 | Whiskey Boot Hill-live (Neil Young) |
| 53 | Expecting To Fly-live (Neil Young) |
| 54 | Cinnamon Girl (Neil Young with Crazy Horse) |
| 55 | Running Dry (Requiem For The Rockets) (Neil Young with Crazy Horse) |
| 56 | Round And Round (It Won't Be Long) (Neil Young with Crazy Horse) |
| 57 | Oh Lonesome Me (Neil Young with Crazy Horse) |
| 58 | Birds [45 RPM Single] [Mono] |
| 59 | Everybody's Alone (Neil Young with Crazy Horse) |
| 60 | I Believe In You (Neil Young with Crazy Horse) |
| 61 | Sea Of Madness (Crosby, Stills, Nash & Young) |
| 62 | Dance Dance Dance (Neil Young with Crazy Horse) |
| 63 | Country Girl |
| 64 | Helpless [Previously Unreleased Mix] |
| 65 | It Might Have Been (Neil Young with Crazy Horse) |
| 66 | Everybody Knows This Is Nowhere [Live At The Filmore East 1970] |
| 67 | Winterlong-live (Neil Young & Crazy Horse) |
| 68 | Down By The River-live (Neil Young & Crazy Horse) |
| 69 | Wonderin'-live (Neil Young & Crazy Horse) |
| 70 | Come On Baby Let's Go Downtown-live (Neil Young & Crazy Horse) |
| 71 | Cowgirl In The Sand-live (Neil Young & Crazy Horse) |
| 72 | Tell Me Why |
| 73 | After The Gold Rush |
| 74 | Only Love Can Break Your Heart |
| 75 | Wonderin' [Previously Unreleased Version] |
| 76 | Don't Let It Bring You Down |
| 77 | Cripple Creek Ferry |
| 78 | Southern Man |
| 79 | Till The Morning Comes |
| 80 | When You Dance, I Can Really Love (Neil Young with Crazy Horse) |
| 81 | Ohio [Stereo 45 RPM Single] |
| 82 | Only Love Can Break Your Heart [Previously Unreleased Live Version] |
| 83 | Tell Me Why [Previously Unreleased Live Version] |
| 84 | Music Is Love (David Crosby, Graham Nash & Neil Young) |
| 85 | See The Sky About To Rain-live (Neil Young) |
| 86 | On The Way Home-live (Neil Young) |
| 87 | Tell Me Why [Live At Massey Hall 1971] |
| 88 | Old Man [Live At Massey Hall 1971] |
| 89 | Journey Through The Past-live (Neil Young) |
| 90 | Helpless [Live At Massey Hall 1971] |
| 91 | Love In Mind [Live At Massey Hall 1971] |
| 92 | A Man Needs A Maid/Heart Of Gold [Suite] [Live At Massey Hall 1971] |
| 93 | Cowgirl In The Sand [Live At Massey Hall 1971] |
| 94 | Don't Let It Bring You Down [Live At Massey Hall 1971] |
| 95 | There's A World [Live At Massey Hall 1971] |
| 96 | Bad Fog Of Loneliness-live (Neil Young) |
| 97 | The Needle And The Damage Done [Live At Massey Hall 1971] |
| 98 | Ohio [Live At Massey Hall 1971] |
| 99 | See The Sky About To Rain [Live At Massey Hall 1971] |
| 100 | Down By The River [Live At Massey Hall 1971] |
| 101 | Dance Dance Dance [Live At Massey Hall 1971] |
| 102 | I Am A Child-live (Neil Young) |
| 103 | Heart Of Gold-live (Neil Young) |
| 104 | The Needle And The Damage Done |
| 105 | Bad Fog Of Loneliness [Previously Unreleased Version] |
| 106 | Old Man (Neil Young with The Stray Gators) |
| 107 | Heart Of Gold |
| 108 | Dance Dance Dance [Previously Unreleased Version] |
| 109 | A Man Needs A Maid [Previously Unreleased Mix] |
| 110 | Harvest (Neil Young with The Stray Gators) |
| 111 | Journey Through The Past [Previously Unreleased Version] |
| 112 | Are You Ready For The Country? (Neil Young with The Stray Gators) |
| 113 | Alabama (Neil Young with The Stray Gators) |
| 114 | Words (Between The Lines Of Age) (Neil Young with The Stray Gators) |
| 115 | Soldier [Previously Unreleased Mix] |
| 116 | War Song [45 RPM Single] [Mono] |